Would changing my CPU multiplier to x9 and gradually bump my clock speed up to 270 and chaging the LTD to x3 help at all?
No, that would not help.
Your running the 166 divider right? So at 240, your RAM is still slightly under 200, at 250, your getting a very slight OC on the RAM, ~207, so I guess it is possible that RAM is an issue, but I doubt it, even the crappiest RAM should take that OC, but you could put a larger divider on it, and see if that is the current limiting factor.
I am still guessing mobo or PSU.....